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10.1073/pnas.1419446112

http://scihub22266oqcxt.onion/10.1073/pnas.1419446112
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C4418885!4418885!25870287
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suck abstract from ncbi


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pmid25870287      Proc+Natl+Acad+Sci+U+S+A 2015 ; 112 (17): 5291-6
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  • Ab initio study of hot electrons in GaAs #MMPMID25870287
  • Bernardi M; Vigil-Fowler D; Ong CS; Neaton JB; Louie SG
  • Proc Natl Acad Sci U S A 2015[Apr]; 112 (17): 5291-6 PMID25870287show ga
  • How does an excited electron lose its energy? This problem is central in fields ranging from condensed matter physics to electrical engineering and chemistry. The cooling of hot electrons in gallium arsenide (GaAs) is the critical process underlying the operation of exciting electronic and optoelectronic devices, but the nature of this cooling is controversial. Here, we present calculations showing that hot electrons in GaAs lose energy chiefly by emitting lattice vibrations. We find a dominant role of acoustic vibrations, challenging the common notion that optical vibrations dominate excited electron energy loss. Our computational approach shines light on microscopic processes that are hard to capture with both experiments and semi-empirical calculations and opens new avenues to compute excited electron dynamics.



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